var dictionary = new Dictionary<string, int>
{
    { "Key", 12 }
};

var aggregateObjectCollection = dictionary.Select(
    entry => new AggregateObject(entry.Key, entry.Value));

迭代字典的最简单形式：

foreach(var item in myDictionary)
{ 
    Console.WriteLine(item.Key);
    Console.WriteLine(item.Value);
}

取决于你是在寻找关键点还是值。。。

来自MSDN Dictionary（TKey，TValue）类描述：

// When you use foreach to enumerate dictionary elements,
// the elements are retrieved as KeyValuePair objects.
Console.WriteLine();
foreach( KeyValuePair<string, string> kvp in openWith )
{
    Console.WriteLine("Key = {0}, Value = {1}", 
        kvp.Key, kvp.Value);
}

// To get the values alone, use the Values property.
Dictionary<string, string>.ValueCollection valueColl =
    openWith.Values;

// The elements of the ValueCollection are strongly typed
// with the type that was specified for dictionary values.
Console.WriteLine();
foreach( string s in valueColl )
{
    Console.WriteLine("Value = {0}", s);
}

// To get the keys alone, use the Keys property.
Dictionary<string, string>.KeyCollection keyColl =
    openWith.Keys;

// The elements of the KeyCollection are strongly typed
// with the type that was specified for dictionary keys.
Console.WriteLine();
foreach( string s in keyColl )
{
    Console.WriteLine("Key = {0}", s);
}

我将利用.NET 4.0+的优势，为最初接受的问题提供更新的答案：

foreach(var entry in MyDic)
{
    // do something with entry.Value or entry.Key
}

如果要使用for循环，可以执行以下操作：

var keyList=new List<string>(dictionary.Keys);
for (int i = 0; i < keyList.Count; i++)
{
    var key= keyList[i];
    var value = dictionary[key];
}

我知道这是一个非常古老的问题，但我创建了一些可能有用的扩展方法：

    public static void ForEach<T, U>(this Dictionary<T, U> d, Action<KeyValuePair<T, U>> a)
    {
        foreach (KeyValuePair<T, U> p in d) { a(p); }
    }

    public static void ForEach<T, U>(this Dictionary<T, U>.KeyCollection k, Action<T> a)
    {
        foreach (T t in k) { a(t); }
    }

    public static void ForEach<T, U>(this Dictionary<T, U>.ValueCollection v, Action<U> a)
    {
        foreach (U u in v) { a(u); }
    }

这样我可以编写如下代码：

myDictionary.ForEach(pair => Console.Write($"key: {pair.Key}, value: {pair.Value}"));
myDictionary.Keys.ForEach(key => Console.Write(key););
myDictionary.Values.ForEach(value => Console.Write(value););