好吧，我来总结一下大家之前说过的话…不管怎样，这是我根据好的答案构建的代码:)剩下要做的就是复制和使用…

/// <summary>
/// Checks to make sure that the input delegate throws a exception of type TException.
/// </summary>
/// <typeparam name="TException">The type of exception expected.</typeparam>
/// <param name="methodToExecute">The method to execute to generate the exception.</param>
public static void AssertRaises<TException>(Action methodToExecute) where TException : System.Exception
{
    try
    {
        methodToExecute();
    }
    catch (TException) {
        return;
    }  
    catch (System.Exception ex)
    {
        Assert.Fail("Expected exception of type " + typeof(TException) + " but type of " + ex.GetType() + " was thrown instead.");
    }
    Assert.Fail("Expected exception of type " + typeof(TException) + " but no exception was thrown.");  
}

对于“Visual Studio Team Test”，似乎您将ExpectedException属性应用到测试的方法。

文档中的示例:使用Visual Studio团队测试的单元测试演练

[TestMethod]
[ExpectedException(typeof(ArgumentException),
    "A userId of null was inappropriately allowed.")]
public void NullUserIdInConstructor()
{
   LogonInfo logonInfo = new LogonInfo(null, "P@ss0word");
}

有一个很棒的库叫做NFluent，它可以加速和简化你编写断言的方式。

编写抛出异常的断言非常简单:

    [Test]
    public void given_when_then()
    {
        Check.ThatCode(() => MethodToTest())
            .Throws<Exception>()
            .WithMessage("Process has been failed");
    }

这是测试方法的一个属性…你不使用Assert。看起来是这样的:

[ExpectedException(typeof(ExceptionType))]
public void YourMethod_should_throw_exception()

如果你使用NUNIT，你可以这样做:

Assert.Throws<ExpectedException>(() => methodToTest());

也可以存储抛出的异常以便进一步验证:

ExpectedException ex = Assert.Throws<ExpectedException>(() => methodToTest());
Assert.AreEqual( "Expected message text.", ex.Message );
Assert.AreEqual( 5, ex.SomeNumber);

参见:http://nunit.org/docs/2.5/exceptionAsserts.html

通常你的测试框架会给出答案。但如果它不够灵活，你可以这样做:

try {
    somethingThatShouldThrowAnException();
    Assert.Fail(); // If it gets to this line, no exception was thrown
} catch (GoodException) { }

正如@Jonas指出的，这并不适用于捕捉基本异常:

try {
    somethingThatShouldThrowAnException();
    Assert.Fail(); // raises AssertionException
} catch (Exception) {
    // Catches the assertion exception, and the test passes
}

如果绝对必须捕获Exception，则需要重新抛出Assert.Fail()。但实际上，这是一个你不应该手写的信号;检查测试框架中的选项，或者查看是否可以抛出更有意义的异常进行测试。

catch (AssertionException) { throw; }

您应该能够根据自己的需要调整这种方法——包括指定要捕获的异常类型。如果你只期望某些类型，完成catch块:

} catch (GoodException) {
} catch (Exception) {
    // not the right kind of exception
    Assert.Fail();
}