最近我不得不在工作中写一些东西来完成这个任务，所以我想我会把我对这个问题的解决方案贴出来。作为一个额外的好处，这个解决方案的功能提供了一种方法，以相反的方向分割字符串，并且它正确地处理上面Marvin Pinto提到的unicode字符。所以，就是这样:

using System;
using Extensions;

namespace TestCSharp
{
    class Program
    {
        static void Main(string[] args)
        {    
            string asciiStr = "This is a string.";
            string unicodeStr = "これは文字列です。";

            string[] array1 = asciiStr.Split(4);
            string[] array2 = asciiStr.Split(-4);

            string[] array3 = asciiStr.Split(7);
            string[] array4 = asciiStr.Split(-7);

            string[] array5 = unicodeStr.Split(5);
            string[] array6 = unicodeStr.Split(-5);
        }
    }
}

namespace Extensions
{
    public static class StringExtensions
    {
        /// <summary>Returns a string array that contains the substrings in this string that are seperated a given fixed length.</summary>
        /// <param name="s">This string object.</param>
        /// <param name="length">Size of each substring.
        ///     <para>CASE: length &gt; 0 , RESULT: String is split from left to right.</para>
        ///     <para>CASE: length == 0 , RESULT: String is returned as the only entry in the array.</para>
        ///     <para>CASE: length &lt; 0 , RESULT: String is split from right to left.</para>
        /// </param>
        /// <returns>String array that has been split into substrings of equal length.</returns>
        /// <example>
        ///     <code>
        ///         string s = "1234567890";
        ///         string[] a = s.Split(4); // a == { "1234", "5678", "90" }
        ///     </code>
        /// </example>            
        public static string[] Split(this string s, int length)
        {
            System.Globalization.StringInfo str = new System.Globalization.StringInfo(s);

            int lengthAbs = Math.Abs(length);

            if (str == null || str.LengthInTextElements == 0 || lengthAbs == 0 || str.LengthInTextElements <= lengthAbs)
                return new string[] { str.ToString() };

            string[] array = new string[(str.LengthInTextElements % lengthAbs == 0 ? str.LengthInTextElements / lengthAbs: (str.LengthInTextElements / lengthAbs) + 1)];

            if (length > 0)
                for (int iStr = 0, iArray = 0; iStr < str.LengthInTextElements && iArray < array.Length; iStr += lengthAbs, iArray++)
                    array[iArray] = str.SubstringByTextElements(iStr, (str.LengthInTextElements - iStr < lengthAbs ? str.LengthInTextElements - iStr : lengthAbs));
            else // if (length < 0)
                for (int iStr = str.LengthInTextElements - 1, iArray = array.Length - 1; iStr >= 0 && iArray >= 0; iStr -= lengthAbs, iArray--)
                    array[iArray] = str.SubstringByTextElements((iStr - lengthAbs < 0 ? 0 : iStr - lengthAbs + 1), (iStr - lengthAbs < 0 ? iStr + 1 : lengthAbs));

            return array;
        }
    }
}

此外，这里还有一个运行此代码结果的图像链接:http://i.imgur.com/16Iih.png

使用正则表达式和Linq:

List<string> groups = (from Match m in Regex.Matches(str, @"\d{4}")
                       select m.Value).ToList();

我觉得这样更有可读性，但这只是个人观点。它也可以是一行代码:)。

static IEnumerable<string> Split(string str, int chunkSize)
{
   IEnumerable<string> retVal = Enumerable.Range(0, str.Length / chunkSize)
        .Select(i => str.Substring(i * chunkSize, chunkSize))

   if (str.Length % chunkSize > 0)
        retVal = retVal.Append(str.Substring(str.Length / chunkSize * chunkSize, str.Length % chunkSize));

   return retVal;
}

它正确地处理不能被chunkSize整除的输入字符串长度。

请注意，可能需要额外的代码来优雅地处理边缘情况(null或空输入字符串，chunkSize == 0)。

static IEnumerable<string> Split(string str, double chunkSize)
{
    return Enumerable.Range(0, (int) Math.Ceiling(str.Length/chunkSize))
       .Select(i => new string(str
           .Skip(i * (int)chunkSize)
           .Take((int)chunkSize)
           .ToArray()));
}

另一种方法是:

using System;
using System.Collections.Generic;
using System.Linq;

public class Program
{
    public static void Main()
    {

        var x = "Hello World";
        foreach(var i in x.ChunkString(2)) Console.WriteLine(i);
    }
}

public static class Ext{
    public static IEnumerable<string> ChunkString(this string val, int chunkSize){
        return val.Select((x,i) => new {Index = i, Value = x})
                  .GroupBy(x => x.Index/chunkSize, x => x.Value)
                  .Select(x => string.Join("",x));
    }
}

static List<string> GetChunks(string value, int chunkLength)
{
    var res = new List<string>();
    int count = (value.Length / chunkLength) + (value.Length % chunkLength > 0 ? 1 : 0);
    Enumerable.Range(0, count).ToList().ForEach(f => res.Add(value.Skip(f * chunkLength).Take(chunkLength).Select(z => z.ToString()).Aggregate((a,b) => a+b)));
    return res;
}

demo

for (int i = 0; i <= Convert.ToInt32(Math.Truncate(Convert.ToDecimal(_string.Length / _chunkSize))); i++)
{
    var _currentChunk = _string.Substring(i * _chunkSize, Math.Min(_chunkSize, _string.Length - i * _chunkSize));
    //do something with current chunk 
}