最好，最简单和一般的答案:)。

    string originalString = "1111222233334444";
    List<string> test = new List<string>();
    int chunkSize = 4; // change 4 with the size of strings you want.
    for (int i = 0; i < originalString.Length; i = i + chunkSize)
    {
        if (originalString.Length - i >= chunkSize)
            test.Add(originalString.Substring(i, chunkSize));
        else
            test.Add(originalString.Substring(i,((originalString.Length - i))));
    }

static List<string> GetChunks(string value, int chunkLength)
{
    var res = new List<string>();
    int count = (value.Length / chunkLength) + (value.Length % chunkLength > 0 ? 1 : 0);
    Enumerable.Range(0, count).ToList().ForEach(f => res.Add(value.Skip(f * chunkLength).Take(chunkLength).Select(z => z.ToString()).Aggregate((a,b) => a+b)));
    return res;
}

demo

for (int i = 0; i <= Convert.ToInt32(Math.Truncate(Convert.ToDecimal(_string.Length / _chunkSize))); i++)
{
    var _currentChunk = _string.Substring(i * _chunkSize, Math.Min(_chunkSize, _string.Length - i * _chunkSize));
    //do something with current chunk 
}

class StringHelper
{
    static void Main(string[] args)
    {
        string str = "Hi my name is vikas bansal and my email id is bansal.vks@gmail.com";
        int offSet = 10;

        List<string> chunks = chunkMyStr(str, offSet);

        Console.Read();
    }

    static List<string> chunkMyStr(string str, int offSet)
    {


        List<string> resultChunks = new List<string>();

        for (int i = 0; i < str.Length; i += offSet)
        {
            string temp = str.Substring(i, (str.Length - i) > offSet ? offSet : (str.Length - i));
            Console.WriteLine(temp);
            resultChunks.Add(temp);


        }

        return resultChunks;
    }
}

根据其他帖子的答案，以及一些使用示例:

public static string FormatSortCode(string sortCode)
{
    return ChunkString(sortCode, 2, "-");
}
public static string FormatIBAN(string iban)
{
    return ChunkString(iban, 4, "  ");
}

private static string ChunkString(string str, int chunkSize, string separator)
{
    var b = new StringBuilder();
    var stringLength = str.Length;
    for (var i = 0; i < stringLength; i += chunkSize)
    {
        if (i + chunkSize > stringLength) chunkSize = stringLength - i;
        b.Append(str.Substring(i, chunkSize));
        if (i+chunkSize != stringLength)
            b.Append(separator);
    }
    return b.ToString();
}

在多芬和康他汀的答案组合中……

static IEnumerable<string> WholeChunks(string str, int chunkSize) {
    for (int i = 0; i < str.Length; i += chunkSize) 
        yield return str.Substring(i, chunkSize);
}

这将适用于所有可以被分割成大量块的字符串，否则将抛出异常。

如果你想支持任意长度的字符串，你可以使用下面的代码:

static IEnumerable<string> ChunksUpto(string str, int maxChunkSize) {
    for (int i = 0; i < str.Length; i += maxChunkSize) 
        yield return str.Substring(i, Math.Min(maxChunkSize, str.Length-i));
}

然而，OP明确表示他不需要这个;它有点长，很难读，稍微慢一点。本着KISS和YAGNI的精神，我选择第一个选项:它可能是最有效的实现，而且非常简短、可读，而且重要的是，它会对不符合规范的输入抛出异常。