List<string> SplitString(int chunk, string input)
{
    List<string> list = new List<string>();
    int cycles = input.Length / chunk;

    if (input.Length % chunk != 0)
        cycles++;

    for (int i = 0; i < cycles; i++)
    {
        try
        {
            list.Add(input.Substring(i * chunk, chunk));
        }
        catch
        {
            list.Add(input.Substring(i * chunk));
        }
    }
    return list;
}

根据其他帖子的答案，以及一些使用示例:

public static string FormatSortCode(string sortCode)
{
    return ChunkString(sortCode, 2, "-");
}
public static string FormatIBAN(string iban)
{
    return ChunkString(iban, 4, "  ");
}

private static string ChunkString(string str, int chunkSize, string separator)
{
    var b = new StringBuilder();
    var stringLength = str.Length;
    for (var i = 0; i < stringLength; i += chunkSize)
    {
        if (i + chunkSize > stringLength) chunkSize = stringLength - i;
        b.Append(str.Substring(i, chunkSize));
        if (i+chunkSize != stringLength)
            b.Append(separator);
    }
    return b.ToString();
}

这也可以用这种方式来完成

        string actualString = "1111222233334444";
        var listResult = new List<string>();
        int groupingLength = actualString.Length % 4;
        if (groupingLength > 0)
            listResult.Add(actualString.Substring(0, groupingLength));
        for (int i = groupingLength; i < actualString.Length; i += 4)
        {
            listResult.Add(actualString.Substring(i, 4));
        }

        foreach(var res in listResult)
        {
            Console.WriteLine(res);
        }
        Console.Read();

List<string> SplitString(int chunk, string input)
{
    List<string> list = new List<string>();
    int cycles = input.Length / chunk;

    if (input.Length % chunk != 0)
        cycles++;

    for (int i = 0; i < cycles; i++)
    {
        try
        {
            list.Add(input.Substring(i * chunk, chunk));
        }
        catch
        {
            list.Add(input.Substring(i * chunk));
        }
    }
    return list;
}

试试这个:

    public static string[] Split(string str, int chunkSize)
    {
        return Enumerable.Range(0, str.Length / chunkSize)
            .Select(i => str.Substring(i * chunkSize, chunkSize)).ToArray();
    }

它基于@dove解决方案，但作为扩展方法实现。

好处:

扩展方法 涵盖角落案例 分割字符串与任何字符:数字，字母，其他符号

Code

public static class EnumerableEx
{    
    public static IEnumerable<string> SplitBy(this string str, int chunkLength)
    {
        if (String.IsNullOrEmpty(str)) throw new ArgumentException();
        if (chunkLength < 1) throw new ArgumentException();

        for (int i = 0; i < str.Length; i += chunkLength)
        {
            if (chunkLength + i > str.Length)
                chunkLength = str.Length - i;

            yield return str.Substring(i, chunkLength);
        }
    }
}

使用

var result = "bobjoecat".SplitBy(3); // bob, joe, cat

为简洁起见，删除了单元测试(请参阅以前的修订版)