我知道这个问题已经有很多年了，但是这里有一个Rx实现。它处理了长度% chunkSize != 0的问题:

   public static IEnumerable<string> Chunkify(this string input, int size)
        {
            if(size < 1)
                throw new ArgumentException("size must be greater than 0");

            return input.ToCharArray()
                .ToObservable()
                .Buffer(size)            
                .Select(x => new string(x.ToArray()))
                .ToEnumerable();
        }

如有必要分割几个不同的长度: 例如，日期和时间的指定格式为stringstrangeStr = "07092016090532";07092016090532(日期:07.09.2016时间:09:05:32)

public static IEnumerable<string> SplitBy(this string str, int[] chunkLength)
    {
        if (String.IsNullOrEmpty(str)) throw new ArgumentException();
        int i = 0;
        for (int j = 0; j < chunkLength.Length; j++)
        {
            if (chunkLength[j] < 1) throw new ArgumentException();
            if (chunkLength[j] + i > str.Length)
            {
                chunkLength[j] = str.Length - i;
            }
            yield return str.Substring(i, chunkLength[j]);
            i += chunkLength[j];
        }
    }

使用:

string[] dt = strangeStr.SplitBy(new int[] { 2, 2, 4, 2, 2, 2, 2 }).ToArray();

最好，最简单和一般的答案:)。

    string originalString = "1111222233334444";
    List<string> test = new List<string>();
    int chunkSize = 4; // change 4 with the size of strings you want.
    for (int i = 0; i < originalString.Length; i = i + chunkSize)
    {
        if (originalString.Length - i >= chunkSize)
            test.Add(originalString.Substring(i, chunkSize));
        else
            test.Add(originalString.Substring(i,((originalString.Length - i))));
    }

这也可以用这种方式来完成

        string actualString = "1111222233334444";
        var listResult = new List<string>();
        int groupingLength = actualString.Length % 4;
        if (groupingLength > 0)
            listResult.Add(actualString.Substring(0, groupingLength));
        for (int i = groupingLength; i < actualString.Length; i += 4)
        {
            listResult.Add(actualString.Substring(i, 4));
        }

        foreach(var res in listResult)
        {
            Console.WriteLine(res);
        }
        Console.Read();

它不是很漂亮，也不是很快，但它是有效的，它是一行程序，它是LINQy:

List<string> a = text.Select((c, i) => new { Char = c, Index = i }).GroupBy(o => o.Index / 4).Select(g => new String(g.Select(o => o.Char).ToArray())).ToList();

根据其他帖子的答案，以及一些使用示例:

public static string FormatSortCode(string sortCode)
{
    return ChunkString(sortCode, 2, "-");
}
public static string FormatIBAN(string iban)
{
    return ChunkString(iban, 4, "  ");
}

private static string ChunkString(string str, int chunkSize, string separator)
{
    var b = new StringBuilder();
    var stringLength = str.Length;
    for (var i = 0; i < stringLength; i += chunkSize)
    {
        if (i + chunkSize > stringLength) chunkSize = stringLength - i;
        b.Append(str.Substring(i, chunkSize));
        if (i+chunkSize != stringLength)
            b.Append(separator);
    }
    return b.ToString();
}